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1 article(s) from Makhloufi, Gamall

The Ugi four-component reaction as a concise modular synthetic tool for photo-induced electron transfer donor-anthraquinone dyads

Sarah Bay,
Gamall Makhloufi,
Christoph Janiak and
Thomas J. J. Müller

Beilstein J. Org. Chem. 2014, 10, 1006–1016, doi:10.3762/bjoc.10.100

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Graphical Abstract

Figure 1: Phenothiazine–anthraquinone dyad 1, donor-only (2) and acceptor-only (3) models assembled by Ugi 4C...

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Scheme 1: Ugi 4CR synthesis of donor–anthraquinone dyads 8.

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Scheme 2: Ugi 4CR synthesis of donor-only reference systems 10.

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Figure 2: Molecular structure of S(O)-1 (left) (30% ellipsoids, except for the CH₃CH₂ end of the hexyl group,...

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Figure 3: Cyclic voltammogram of dyad 8c (recorded in CH₂Cl₂, T = 298 K, c (8c) = 0.1 mol·L⁻¹, Pt working ele...

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Figure 4: DFT-computed (B3LYP, 6-311G*) frontier molecular orbitals HOMO (bottom) and LUMO (top) of the pheno...

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Figure 5: Normalized absorption spectra of the phenothiazine–anthraquinone dyad 8c (recorded in CH₂Cl₂, c (8c...

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Figure 6: Absorption spectra of Do–anthraquinone dyads 8c (top) and 8e (bottom) with the corresponding refere...

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Figure 7: Normalized absorption and emission spectra of Ugi-donor compounds 2 and 10 (recorded in CH₂Cl₂, T =...

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Figure 8: Emission spectra of donor-only system 2 phenothiazine–anthraquinone dyads 8a,b (top), and the donor...

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Published 05 May 2014

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